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Direct Determination of the Effect of Strain on Domain Morphology in Ferroelectric Superlattices with Scanning Probe Microscopy

机译:扫描探针显微镜直接确定应变对铁电超晶格畴形态的影响

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摘要

A variant of piezo force microscopy was used to characterize the effect of strain on polarization in [(BaTiO3)n/(SrTiO3)m]p superlattices. The measurements were compared to theoretical predictions based on phase-field calculations. When polarization is constrained to be perpendicular to the substrate, the measured polarization and domain morphology agree quantitatively with the predictions. This case allows the presence of an internal electric field in the thin film to be identified. The measured trend in piezoelectric response with strain state was in qualitative agreement with predictions, and the differences were consistent with the presence of internal electrical fields. Clear differences in domain morphology with strain were observed; and in some cases, the lateral anisotropic strain appeared to influence the domain morphology. The differences in magnitude and morphology were attributed to the internal electric fields and anisotropic strains.
机译:使用压电力显微镜的变体来表征应变对[(BaTiO3)n /(SrTiO3)m] p超晶格中的极化的影响。将测量结果与基于相场计算的理论预测进行比较。当极化被限制为垂直于基板时,所测得的极化和畴形态在定量上与预测一致。这种情况允许识别薄膜中存在内部电场。应变状态下压电响应的测量趋势与预测定性一致,差异与内部电场的存在一致。观察到域形态随应变的明显差异;在某些情况下,横向各向异性应变似乎会影响畴的形态。大小和形态的差异归因于内部电场和各向异性应变。

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